Physics – Condensed Matter – Strongly Correlated Electrons
Scientific paper
2010-03-23
Physica Status Solidi B 247, 671 (2010)
Physics
Condensed Matter
Strongly Correlated Electrons
5 pages, 6 figures, published in Physica Status Solidi B
Scientific paper
10.1002/pssb.200983077
The S=1/2 antiferromagnetic Heisenberg chain exhibits a magnetic field driven quantum critical point. We study the low frequency spin dynamics in copper pyrazine dinitrate (CuPzN), a realization of this model system of quantum magnetism, by means of $^{13}$C-NMR spectroscopy. Measurements of the nuclear spin-lattice relaxation rate $T_1^{-1}$ in the vicinity of the saturation field are compared with quantum Monte Carlo calculations of the dynamic structure factor. Both show a strong divergence of low energy excitations at temperatures in the quantum regime. The analysis of the anisotropic $T_1^{-1}$-rates and frequency shifts allows one to disentangle the contributions from transverse and longitudinal spin fluctuations for a selective study and to determine the transfer of delocalized spin moments from copper to the neighboring nitrogen atoms.
Brenig Wolfram
Grossjohann Simon
Guenther M. M.
Klauss Hans-Henning
Kuehne Heiko
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