Physics – Condensed Matter – Strongly Correlated Electrons
Scientific paper
2011-03-29
Phys. Rev. Lett. 107, 107403 (2011)
Physics
Condensed Matter
Strongly Correlated Electrons
Scientific paper
10.1103/PhysRevLett.107.107403
We report inelastic x-ray scattering measurements of the temperature dependence of phonon dispersion in the prototypical charge-density-wave (CDW) compound NbSe2. Surprisingly, acoustic phonons soften to zero frequency and become overdamped over an extended region around the CDW wavevector. This extended phonon collapse is dramatically different from the sharp cusp in the phonon dispersion expected from Fermi surface nesting. Instead, our experiments combined with ab initio calculations, show that it is the wavevector dependence of the electron-phonon coupling that drives the CDW formation in NbSe$_2$ and determines its periodicity. This mechanism explains the so far enigmatic behavior of CDW in NbSe$_2$ and may provide a new approach to other strongly correlated systems where electron-phonon coupling is important.
Bohnen Klaus Peter
Castellan John-Paul
Egami Takeshi
Heid Rolf
Hott Roland
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