Physics – Condensed Matter
Scientific paper
2003-05-10
Physics
Condensed Matter
5 pages, 4 figure. To be published in Phys. Rev. B
Scientific paper
10.1103/PhysRevB.67.212202
We describe a simple model for the melting and optical properties of a DNA/gold nanoparticle aggregate. The optical properties at fixed wavelength change dramatically at the melting transition, which is found to be higher and narrower in temperature for larger particles, and much sharper than that of an isolated DNA link. All these features are in agreement with available experiments. The aggregate is modeled as a cluster of gold nanoparticles on a periodic lattice connected by DNA bonds, and the extinction coefficient is computed using the discrete dipole approximation. Melting takes place as an increasing number of these bonds break with increasing temperature. The melting temperature corresponds approximately to the bond percolation threshold.
Park Sung Yong
Stroud David
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