Physics – Condensed Matter – Mesoscale and Nanoscale Physics
Scientific paper
2011-05-05
Nano Lett., 11 (11), pp 4688-4692 (2011)
Physics
Condensed Matter
Mesoscale and Nanoscale Physics
4 pgs, 2 fgs
Scientific paper
10.1021/nl202318u
Strong electron-electron interactions in graphene are expected to result in multiple-excitation generation by the absorption of a single photon. We show that the impact of carrier multiplication on photocurrent response is enhanced by very inefficient electron cooling, resulting in an abundance of hot carriers. The hot-carrier-mediated energy transport dominates the photoresponse and manifests itself in quantum efficiencies that can exceed unity, as well as in a characteristic dependence of the photocurrent on gate voltages. The pattern of multiple photocurrent sign changes as a function of gate voltage provides a fingerprint of hot-carrier-dominated transport and carrier multiplication.
Levitov Leonid S.
Marcus Charles M.
Rudner Mark S.
Song Justin C. W.
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