Influence of electron correlations on ground-state properties of III-V semiconductors

Physics – Condensed Matter – Materials Science

Scientific paper

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4 pages, Latex, no figures, Phys. Rev. B, accepted

Scientific paper

10.1103/PhysRevB.55.4027

Lattice constants and bulk moduli of eleven cubic III-V semiconductors are calculated using an ab initio scheme. Correlation contributions of the valence electrons, in particular, are determined using increments for localized bonds and for pairs and triples of such bonds; individual increments, in turn, are evaluated using the coupled cluster approach with single and double excitations. Core-valence correlation is taken into account by means of a core polarization potential. Combining the results at the correlated level with corresponding Hartree-Fock data, we obtain lattice constants which agree with experiment within an average error of -0.2%; bulk moduli are accurate to +4%. We discuss in detail the influence of the various correlation contributions on lattice constants and bulk moduli.

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