Physics – Condensed Matter – Strongly Correlated Electrons
Scientific paper
2011-11-18
Phys. Rev. B 85, 104416 (2012)
Physics
Condensed Matter
Strongly Correlated Electrons
14 pages, 12 figures, new figures added, final version
Scientific paper
10.1103/PhysRevB.85.104416
Motivated by experiments on non-magnetic triangular-lattice Mott insulators, we study one candidate paramagnetic phase, the columnar dimer (or valence-bond) phase. We apply variants of the bond-operator theory to a dimerized and spatially anisotropic spin-1/2 Heisenberg model and determine its zero-temperature phase diagram and the spectrum of elementary triplet excitations (triplons). Depending on model parameters, we find that the minimum of the triplon energy is located at either a commensurate or an incommensurate wavevector. Condensation of triplons at this commensurate-incommensurate transition defines a quantum Lifshitz point, with effective dimensional reduction which possibly leads to non-trivial paramagnetic (e.g. spin-liquid) states near the closing of the triplet gap. We also discuss the two-particle decay of high-energy triplons, and we comment on the relevance of our results for the organic Mott insulator EtMe3P[Pd(dmit)2]2.
Doretto R. L.
Vojta Matthias
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