Statistical Mechanics of Splay Flexoelectricity in Nematic Liquid Crystals

Details Statistical Mechanics of Splay Flexoelectricity in Nematic Liquid Crystals Statistical Mechanics of Splay Flexoelectricity in Nematic Liquid Crystals

2009-11-10

arxiv.org/abs/0911.1991v1

Phys. Rev. E 81, 031704 (2010)

Physics

Condensed Matter

Soft Condensed Matter

8 pages, including 15 postscript figures, uses REVTeX 4

Scientific paper

10.1103/PhysRevE.81.031704

We develop a lattice model for the splay flexoelectric effect in nematic liquid crystals. In this model, each lattice site has a spin representing the local molecular orientation, and the interaction between neighboring spins represents pear-shaped molecules with shape polarity. We perform Monte Carlo simulations and mean-field calculations to find the behavior as a function of interaction parameters, temperature, and applied electric field. The resulting phase diagram has three phases: isotropic, nematic, and polar. In the nematic phase, there is a large splay flexoelectric effect, which diverges as the system approaches the transition to the polar phase. These results show that flexoelectricity is a statistical phenomenon associated with the onset of polar order.

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