Raman scattering for triangular lattices spin-1/2 Heisenberg antiferromagnets

Physics – Condensed Matter – Strongly Correlated Electrons

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To appear in J. of Phys. Condens. Matter (Proceedings of International Conference "Highly Frustrated Magnets", Osaka (Japan),

Scientific paper

Motivated by various spin-1/2 compounds like Cs$_2$CuCl$_4$ or $\kappa$-(BEDT-TTF)$_2$Cu$_2$(CN)$_3$, we derive a Raman-scattering operator {\it \`a la} Shastry and Shraiman for various geometries. For T=0, the exact spectra is computed by Lanczos algorithm for finite-size clusters. We perform a systematic investigation as a function of $J_2/J_1$, the exchange constant ratio: ranging from $J_2=0$, the well known square-lattice case, to $J_2/J_1=1$ the isotropic triangular lattice. We discuss the polarization dependence of the spectra and show how it can be used to detect precursors of the instabilities of the ground state against quantum fluctuations.

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