Light Quasiparticles Dominate Electronic Transport in Molecular Crystal Field-Effect Transistors

Details Light Quasiparticles Dominate Electronic Transport in Molecular Crystal Field-Effect Transistors Light Quasiparticles Dominate Electronic Transport in Molecular Crystal Field-Effect Transistors

2007-07-11

arxiv.org/abs/0707.1604v1

Phys. Rev. Lett. 99, 016403 (2007)

Physics

Condensed Matter

Materials Science

4 pages, 4 figures

Scientific paper

10.1103/PhysRevLett.99.016403

We report on an infrared spectroscopy study of mobile holes in the accumulation layer of organic field-effect transistors based on rubrene single crystals. Our data indicate that both transport and infrared properties of these transistors at room temperature are governed by light quasiparticles in molecular orbital bands with the effective masses m* comparable to free electron mass. Furthermore, the m* values inferred from our experiments are in agreement with those determined from band structure calculations. These findings reveal no evidence for prominent polaronic effects, which is at variance with the common beliefs of polaron formation in molecular solids.

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