Theoretical and numerical studies of chemisorption on a line with precursor layer diffusion

Details Theoretical and numerical studies of chemisorption on a line with precursor layer diffusion Theoretical and numerical studies of chemisorption on a line with precursor layer diffusion

1995-08-10

arxiv.org/abs/cond-mat/9508039v1

Physics

Condensed Matter

17 pages(LaTeX), 11 figures(1 PS file, uuencoded), submmited to Phys. Rev. E

Scientific paper

10.1103/PhysRevE.52.6044

We consider a model for random deposition of monomers on a line with extrinsic precursor states. As the adsorbate coverage increases, the system develops non-trivial correlations due to the diffusion mediated deposition mechanism. In a numeric simulation, we study various quantities describing the evolution of the island structure. We propose a simple, self-consistent theory which incorporates pair correlations. The results for the correlations, island density number, average island size and probabilities of island nucleation, growth and coagulation show good agreement with the simulation data.

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