Photon Counting Statistics for Single Molecule Spectroscopy

Details Photon Counting Statistics for Single Molecule Spectroscopy Photon Counting Statistics for Single Molecule Spectroscopy

2001-04-11

arxiv.org/abs/cond-mat/0104188v1

Physics

Condensed Matter

Statistical Mechanics

Scientific paper

We present a general relation between Mandel's $Q$ parameter describing
variance of number of photons emitted from a single molecule and a three time
correlation function describing a spectral diffusion process the molecule is
undergoing. For a prototype of such a stochastic process an exact solution is
found which exhibits rich types of physical behaviors.

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