Physics – Condensed Matter – Statistical Mechanics
Scientific paper
1998-07-06
Phys. Rev. B 58 (Rapid Comm.), No. 22, R14 733 - R14736 (1 December 1998-II)
Physics
Condensed Matter
Statistical Mechanics
REVTeX, 3 pages, 6 figures (postscript)
Scientific paper
10.1103/PhysRevB.58.R14733
A new type of mesoscopic quantum effect in large-spin molecules possessing easy-axis anisotropy, such as Mn12, is predicted. The response of such a system to an external field applied perpendicular to the easy axis is considered. It is shown that the susceptibility of this system exhibits a peculiar peak of purely quantum origin. This effect arises from very general properties of quantum fluctuations in spin systems. We demonstrate that the effect is entirely accessible for contemporary experimental techniques. Our studies show that the many-spin nature of the Mn12 clusters is important for a correct description of this quantum peak.
Dobrovitski Viatcheslav V.
Harmon Bruce N.
Katsnelson Mikhail I.
Zvezdin Anatolii K.
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