Structural properties and optical response of Na clusters in Ne, Ar, and Kr matrices

Details Structural properties and optical response of Na clusters in Ne, Ar, and Kr matrices Structural properties and optical response of Na clusters in Ne, Ar, and Kr matrices

2007-06-14

arxiv.org/abs/0706.2119v1

Phys. Rev. B 75, 235418 (2007)

Physics

Condensed Matter

Other Condensed Matter

9 pages, 3 figures, 1 table accepted in Phys. Rev. B

Scientific paper

10.1103/PhysRevB.75.235418

We discuss the structural properties and optical response of a small Na cluster inside rare gas (RG) matrices of Ne, Ar, or Kr atoms. The mixed systems are described with a hierarchical model, treating the cluster at a quantum mechanical level and the matrix atoms classically in terms of their positions and polarizations. We pay special attention to the differences caused by the different matrix types. These differences can be explained by the interplay of core repulsion and dipole attraction in the interaction between the cluster electrons and the RG atoms.

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