Physics – Condensed Matter – Strongly Correlated Electrons
Scientific paper
2008-07-25
EPL, 86 (2009) 37004
Physics
Condensed Matter
Strongly Correlated Electrons
4+x pages, 2 figures
Scientific paper
10.1209/0295-5075/86/37004
Materials with strong electronic Coulomb interactions play an increasing role in modern materials applications. "Thermochromic" systems, which exhibit thermally induced changes in their optical response, provide a particularly interesting case. The optical switching associated with the metal-insulator transition of vanadium dioxide (VO2), for example, has been proposed for use in "intelligent" windows, which selectively filter radiative heat in hot weather conditions. In this work, we develop the theoretical tools for describing such a behavior. Using a novel scheme for the calculation of the optical conductivity of correlated materials, we obtain quantitative agreement with experiments for both phases of VO2. On the example of an optimized energy-saving window setup, we further demonstrate that theoretical materials design has now come into reach, even for the particularly challenging class of correlated electron systems.
Biermann Silke
Tomczak Jan M.
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