Physics – Condensed Matter
Scientific paper
1996-05-14
PRL 78, 1066 (1997)
Physics
Condensed Matter
Replaced with the final text, accepted for publication in PRL. 1 Fig. added. Misc. text revisions
Scientific paper
10.1103/PhysRevLett.78.1066
We present a unified view of orientational ordering in phases I, II, and III of solid hydrogen. Phases II and III are orientationally ordered, while the ordering objects in phase II are angular momenta of rotating molecules, and in phase III the molecules themselves. This concept provides quantitative explanation of the vibron softening, libron and roton spectra, and increase of the IR vibron oscillator strength in phase III. The temperature dependence of the effective charge parallels the frequency shifts of the IR and Raman vibrons. All three quantities are linear in the order parameter.
Goncharov Alexander F.
Hanfland Michael
Hemley Russell J.
Mao H.-K.
Mazin Igor I.
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