Nonlinear optical response in higher fullerenes

Details Nonlinear optical response in higher fullerenes Nonlinear optical response in higher fullerenes

1997-02-20

arxiv.org/abs/cond-mat/9702181v1

Jpn. J. Appl. Phys. 36 (1997) L485-L487

Physics

Condensed Matter

Condensed Matter Theory Group at ETL: http://www.etl.go.jp/Organization/Bussei-kiso/

Scientific paper

10.1143/JJAP.36.L485

Nonlinear optical properties of extracted higher fullerenes - C70, C76, C78, and C84 - are theoretically investigated. Magnitudes of off-resonant third-harmonic-generation are calculated by the intermediate exciton theory. We find that optical nonlinearities of higher fullerenes are a few times larger than those of C60. The magnitudes of nonlinearity tend to increase as the optical gap decreases in higher fullerenes.

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