Physics – Condensed Matter – Mesoscale and Nanoscale Physics
Scientific paper
2005-05-16
Physics
Condensed Matter
Mesoscale and Nanoscale Physics
Significantly different content -- inadequacy of SCF approach described with simple model, and a whole new class of experiment
Scientific paper
10.1103/PhysRevB.73.155410
We identify experimental signatures in the current-voltage (I-V) characteristics of weakly contacted molecules directly arising from excitations in their many electron spectrum. The current is calculated using a multielectron master equation in the Fock space of an exact diagonalized model many-body Hamiltonian for a prototypical molecule. Using this approach, we explain several nontrivial features in frequently observed I-Vs in terms of a rich spectrum of excitations that may be hard to describe adequately with standard one-electron self-consistent field (SCF) theories.
Datta Saiti
Ghosh Avik W.
Muralidharan Bhaskaran
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