Physics – Condensed Matter – Strongly Correlated Electrons
Scientific paper
2007-08-02
Physical Review Letters Vol.100, 206401 (2008)
Physics
Condensed Matter
Strongly Correlated Electrons
4 pages, 3 figures
Scientific paper
10.1103/PhysRevLett.100.206401
We have re-examined the valence-band (VB) and core-level electronic structure of NiO by means of hard and soft x-ray photoemission spectroscopy (PES). The spectral weight of the lowest energy state found to be enhanced in the bulk sensitive Ni 2p core-level PES. A configuration-interaction model including the bound state screening has shown significant agreement with the core-level spectra, and the off and on-resonance VB spectra. These results identify the lowest energy state in core-level and VB-PES as the Zhang-Rice doublet bound state, consistent with the spin-fermion model and recent ab initio calculation with dynamical mean-field theory (LDA + DMFT).
Chainani Ashish
Eguchi R.
Ishida Yasuchika
Ishikawa Tadashi
Matsunami Masaharu
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