Role of three-body interactions in formation of bulk viscosity in liquid argon

Details Role of three-body interactions in formation of bulk viscosity in liquid argon Role of three-body interactions in formation of bulk viscosity in liquid argon

2012-04-05

arxiv.org/abs/1204.1235v1

J. Chem. Phys. 136 (2012) 164501

Physics

Condensed Matter

Soft Condensed Matter

4 pages, 3 figures

Scientific paper

10.1063/1.4704930

With the aim of locating the origin of discrepancy between experimental and computer simulation results on bulk viscosity of liquid argon, a molecular dynamic simulation of argon interacting via ab initio pair potential and triple-dipole three-body potential has been undertaken. Bulk viscosity, obtained using Green-Kubo formula, is different from the values obtained from modeling argon using Lennard-Jones potential, the former being closer to the experimental data. The conclusion is made that many-body inter-atomic interaction plays a significant role in formation of bulk viscosity.

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