Transport and optical response of molecular junctions driven by surface plasmon-polaritons

Details Transport and optical response of molecular junctions driven by surface plasmon-polaritons Transport and optical response of molecular junctions driven by surface plasmon-polaritons

2009-11-12

arxiv.org/abs/0911.2499v1

Phys. Rev. B 81, 165307 (2010).

Physics

Condensed Matter

Mesoscale and Nanoscale Physics

9 pages, 6 figures

Scientific paper

10.1103/PhysRevB.81.165307

We consider a biased molecular junction subjected to external time-dependent electromagnetic field. The field for two typical junction geometries (bowtie antennas and metal nanospheres) is calculated within finite-difference time-domain technique. Time-dependent transport and optical response of the junctions is calculated within non-equilibrium Green's function approach expressed in a form convenient for description of multi-level systems. We present numerical results for a two-level (HOMO-LUMO) model, and discuss influence of localized surface plasmon polariton modes on transport.

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