Molecular Dynamics Study of the Primary Ferrofluid Aggregate Formation

Details Molecular Dynamics Study of the Primary Ferrofluid Aggregate Formation Molecular Dynamics Study of the Primary Ferrofluid Aggregate Formation

2011-12-16

arxiv.org/abs/1112.4431v2

Physics

Condensed Matter

Materials Science

Submitted to JMMM

Scientific paper

Investigations of the phase transitions and self-organization in the magnetic aggregates are of the fundamental and applied interest. The long-range ordering structures described in the Tom\'anek's systematization (M. Yoon, and D. Tom\'anek, 2010 [1]) are not yet obtained in the direct molecular dynamics simulations. The result structures usually are the linear chains or circles, or, else, amorphous (liquid) formations. In the present work, it was shown, that the thermodynamically equilibrium primary ferrofluid aggregate has either the long-range ordered or liquid phase. Due to the unknown steric layer force and other model idealizations, the clear experimental verification of the real equilibrium phase is still required. The predicted long-range ordered (crystallized) phase produces the faceting shape of the primary ferrofluid aggregate, which can be recognized experimentally. Dynamic formation of all observed ferrofluid nanostructures conforms to the Tom\'anek's systematization.

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