Kinetic description of diffusion-limited reactions in random catalytic media

Details Kinetic description of diffusion-limited reactions in random catalytic media Kinetic description of diffusion-limited reactions in random catalytic media

1997-10-10

arxiv.org/abs/cond-mat/9710099v1

J. Chem. Phys. 108, 1140 (1998)

Physics

Condensed Matter

15 pages, Latex, two figures, to appear in J. Chem. Phys

Scientific paper

10.1063/1.475476

We study the kinetics of bimolecular, catalytically-activated reactions (CARs) in d-dimensions. The elementary reaction act between reactants takes place only when these meet in the vicinity of a catalytic site; such sites are assumed to be immobile and randomly distributed in space. For CARs we develop a kinetic formalism, based on Collins-Kimball-type ideas; within this formalism we obtain explicit expressions for the effective reaction rates and for the decay of the reactants' concentrations.

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