Physics – Condensed Matter – Mesoscale and Nanoscale Physics
Scientific paper
2009-11-12
Phys. Rev. Lett. 104, 177401 (2010)
Physics
Condensed Matter
Mesoscale and Nanoscale Physics
5 pages, 4 figures, final version
Scientific paper
10.1103/PhysRevLett.104.177401
We report a femtosecond mid-infrared study of the broadband low-energy response of individually separated (6,5) and (7,5) single-walled carbon nanotubes. Strong photoinduced absorption is observed around 200 meV, whose transition energy, oscillator strength, resonant chirality enhancement and dynamics manifest the observation of quasi-1D intra-excitonic transitions. A model of the nanotube 1s-2p cross section agrees well with the signal amplitudes. Our study further reveals saturation of the photoinduced absorption with increasing phase-space filling of the correlated e-h pairs.
Fleming Graham R.
Graham Matt W.
Kaindl Robert A.
Ma Yingzhong
Wang Jigang
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