Physics – Condensed Matter – Materials Science
Scientific paper
2005-06-07
Physics
Condensed Matter
Materials Science
Revised text
Scientific paper
10.1117/12.615443
We measure nonlinear optical scattering from individual Au nanorods excited by ultrafast laser pulses on resonance with their longitudinal plasmon mode. Isolating single rods removes inhomogeneous broadening and allows the measurement of a large nonlinearity, much greater than that of nanorod ensembles. Surprisingly, the ultrafast nonlinearity can be attributed entirely to heating of conduction electrons and does not exhibit any response associated with coherent plasmon oscillation. This indicates a previously unobserved damping of strongly driven plasmons.
Guyot-Sionnest Philippe
Liu Mingzhao
Park Sungnam
Pelton Matthew
Scherer Norbert F.
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