Physics – Condensed Matter – Other Condensed Matter
Scientific paper
2008-06-17
Physics
Condensed Matter
Other Condensed Matter
8 pages, 3 figures
Scientific paper
10.1063/1.2977463
Ultrafast degenerate pump-probe experiments performed on a free standing film of double walled carbon nanotubes near the first metallic transition energy of outer tube show ultrafast ($97 fs$) photobleaching followed by a photo-induced absorption with a slow relaxation of $1.8 ps$. Femtosecond closed and open aperture z-scan experiments carried out at the same excitation energy show saturation absorption and negative cubic nonlinearity. From these measurements, real and imaginary part of the third order nonlinear susceptibility are estimated to be Re($\chi^{(3)}) \sim -2.2 \times 10 ^{-9} esu$ and Im($\chi^{(3)}) \sim 1.1 \times 10 ^{-11} esu$.
Kamaraju N.
Karthikeyan B.
Kumar Sunil
Loutfy Raouf O.
Moravsky Alexander
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