Translation-Rotation Coupling in Transient Grating Experiments : Theoretical and Experimental Evidences

Details Translation-Rotation Coupling in Transient Grating Experiments : Theoretical and Experimental Evidences Translation-Rotation Coupling in Transient Grating Experiments : Theoretical and Experimental Evidences

2001-06-29

arxiv.org/abs/cond-mat/0106632v2

Physics

Condensed Matter

Disordered Systems and Neural Networks

PDF format, 14 pages including 4 figures, accepted for publication in EPL. minor modifications

Scientific paper

10.1209/epl/i2001-00533-6

The results of a Transient Grating experiment in a supercooled molecular liquid of anisotropic molecules and its theoretical interpretation are presented. These results show the existence of two distinct dynamical contributions in the response function of this experiment, density and orientation dynamics. These dynamics can be experimentally disentangled by varying the polarisation of the probe and diffracted beams and they have been identified and measured in a Heterodyne Detected experiment performed on m-toluidine. The results of the theory show a good qualitative agreement with the measurements at all temperatures.

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