Thermoelectric properties of electrically gated bismuth telluride nanowires

Details Thermoelectric properties of electrically gated bismuth telluride nanowires Thermoelectric properties of electrically gated bismuth telluride nanowires

2009-08-05

arxiv.org/abs/0908.0624v2

Phys. Rev. B 81, 075316 (2010)

Physics

Condensed Matter

Mesoscale and Nanoscale Physics

19 pages, 12 figures, added references, added 2 tables, removed figures 7,8,9, added new fig. 8

Scientific paper

10.1103/PhysRevB.81.075316

We theoretically studied the effect of the perpendicular electric field on the thermoelectric properties of the intrinsic, n-type and p-type bismuth telluride nanowires with the growth direction [110]. The electronic structure and the wave functions were calculated by solving self-consistently the system of the Schrodinger and Poisson equations using the spectral method. The Poisson equation was solved in terms of the Newton - Raphson method within the predictor-corrector approach. The electron - electron exchange - correlation interactions were taken into account in our analysis. In the temperature range from 77 to 500 K, the dependences of the Seebeck coefficient, thermal conductivity, electron (hole) concentration, and thermoelectric figure of merit on the nanowire thickness, gate voltage, and excess hole (electron) concentration were investigated in the constant relaxation-time approximation. The results of our calculations indicate that the external perpendicular electric field can increase the Seebeck coefficient of the bismuth telluride nanowires with thicknesses of 7 - 15 nm by nearly a factor of 2 and enhance ZT by an order of magnitude. At room temperature, ZT can reach a value as high as 3.4 under the action of the external perpendicular electric field for realistic widths of the nanowires. The obtain results may open up a completely new way for a drastic enhancement of the thermoelectric figure of merit in a wide temperature range.

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