Physics – Condensed Matter
Scientific paper
1996-09-10
Phys. Rev. B 54 (1996) 17452
Physics
Condensed Matter
15 pages, 5 PostScript figures, submitted to Physical Review B
Scientific paper
10.1103/PhysRevB.54.17452
We present a theory of the linear and nonlinear optical characteristics of the insulating phase of the Falicov-Kimball model within the self-consistent mean-field approximation. The Coulomb attraction between the itinerant d-electrons and the localized f-holes gives rise to a built-in coherence between the d and f-states, which breaks the inversion symmetry of the underlying crystal, leading to: (1) electronic ferroelectricity, (2) ferroelectric resonance, and (3) a nonvanishing susceptibility for second-harmonic generation. As experimental tests of such a built-in coherence in mixed-valent compounds we propose measurements of the static dielectric constant, the microwave absorption spectrum, and the dynamic second-order susceptibility.
Ostreich Th.
Portengen T.
Sham L. J.
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