Supercooled Water and the Kinetic Glass Transition II: Collective Dynamics

Details Supercooled Water and the Kinetic Glass Transition II: Collective Dynamics Supercooled Water and the Kinetic Glass Transition II: Collective Dynamics

1997-06-05

arxiv.org/abs/cond-mat/9706039v1

Physics

Condensed Matter

Soft Condensed Matter

rev-tex + 9 figures

Scientific paper

10.1103/PhysRevE.56.5397

In this article we study in detail the Q-vector dependence of the collective dynamics in simulated deeply supercooled SPC/E water. The evolution of the system has been followed for 250 ns at low T, allowing a clear identification of a two step relaxation process. We present evidence in favor of the use of the mode coupling theory for supercooled liquid as framework for the description of the slow alpha-relaxation dynamics in SPC/E water, notwithstanding the fact that the cage formation in this system is controlled by the formation of an open network of hydrogen bonds as opposed to packing constraints, as in the case of simple liquids.

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