Strong ferromangnetism and weak antiferroamgnetism in double perovskites: Sr$_2$Fe{/it M}O$_6$ ({/it M}=Mo, W and Re)

Details Strong ferromangnetism and weak antiferroamgnetism in double perovskites: Sr$_2$Fe{/it M}O$_6$ ({/it M}=Mo, W and Re) Strong ferromangnetism and weak antiferroamgnetism in double perovskites: Sr$_2$Fe{/it M}O$_6$ ({/it M}=Mo, W and Re)

2001-03-08

arxiv.org/abs/cond-mat/0103189v1

Phys. Rev. B 63, 180407 (2001).

Physics

Condensed Matter

Materials Science

4 pages, 3 figures; accepted by PRB as rapid communication

Scientific paper

10.1103/PhysRevB.63.180407

Double perovskites Sr$_2$FeMO$_6$ (M=Mo and Re) exhibit significant colossal magnetoresistance even at room temperature due to the high Curie Temperature (419K and 401K). However, such a high Curie Temperature is puzzling, given the large separation between magnetic elements (Fe). Moreover, with M=W, the electronic and magnetic properties suddenly change to insulating and antiferromagnetic with the N{\'e}el temperature of only 16$\sim$37 K. Based on detailed electronic structure calculations, a new mechanism is proposed which stabilizes the strong ferromagnetic state for M=Mo and Re and is passivated for M=W.

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