Spectral functions of isolated Ce adatoms on paramagnetic surfaces

Details Spectral functions of isolated Ce adatoms on paramagnetic surfaces Spectral functions of isolated Ce adatoms on paramagnetic surfaces

2011-02-16

arxiv.org/abs/1102.3397v1

Phys. Rev. Lett. 107, 026801 (2011)

Physics

Condensed Matter

Strongly Correlated Electrons

4 pages, 3 figures

Scientific paper

10.1103/PhysRevLett.107.026801

We report photoemission experiments revealing the full valence electron spectral function of Ce adatoms on Ag(111), W(110) and Rh(111) surfaces. A transfer of Ce 4f spectral weight from the ionization peak towards the Fermi level is demonstrated upon changing the substrate from Ag(111) to Rh(111). In the intermediate case of Ce on W(110) the ionization peak is found to be split. This evolution of the spectra is explained by means of first-principles theory which clearly demonstrates that a reliable understanding of magnetic adatoms on metal surfaces requires simultaneous low and high energy spectroscopic information.

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