Physics – Condensed Matter – Statistical Mechanics
Scientific paper
1997-09-29
J. Electrochem. Soc. 146, 1035 (1999).
Physics
Condensed Matter
Statistical Mechanics
16 pages, to appear in J Electrochem Soc. Simulation MPEG movies at http://www.scri.fsu.edu/~rikvold
Scientific paper
Numerical studies of lattice-gas models are well suited to describe multi-adsorbate systems. One example is the underpotential deposition of Cu on Au(111) in the presence of sulfuric acid. Preliminary results from dynamic Monte Carlo simulations of the evolution of the adsorbed layer during potential-step experiments across phase transitions are presented for this particular system. The simulated current profiles reproduce a strong asymmetry seen in recent experiments. Examination of the microscopic structures that occur during the simulated evolution processes raises questions that need to be investigated by further experimental and theoretical study.
Brown Gregory
Novotny Mark A.
Rikvold Per Arne
Wieckowski Andrzej
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