Physics – Condensed Matter – Mesoscale and Nanoscale Physics
Scientific paper
2003-02-28
PRB 68, 115105 (2003)
Physics
Condensed Matter
Mesoscale and Nanoscale Physics
8 pages
Scientific paper
10.1103/PhysRevB.68.115105
We consider electrical transport through single molecules coupled to metal electrodes via tunneling barriers. Approximating the molecule by the Anderson impurity model as the simplest model which includes Coulomb charging effects, we extend the ``orthodox'' theory to expand current and shot noise systematically order by order in the tunnel couplings. In particular, we show that a combined measurement of current and shot noise reveals detailed information of the system even in the weak-coupling limit, such as the ratio of the tunnel-coupling strengths of the molecule to the left and right electrode, and the presence of the Coulomb charging energy. Our analysis holds for single-level quantum dots as well.
Hettler Matthias H.
Konig Jurgen
Schön Gerd
Thielmann Axel
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