Selection of dominant multi-exciton transitions in disordered linear J-aggregates

Details Selection of dominant multi-exciton transitions in disordered linear J-aggregates Selection of dominant multi-exciton transitions in disordered linear J-aggregates

2007-07-05

arxiv.org/abs/0707.0826v1

J. Lumin.128, 945 (2008)

Physics

Condensed Matter

Disordered Systems and Neural Networks

8 pages, 2 figures, accepted to Journal of Luminescence

Scientific paper

10.1016/j.jlumin.2007.11.052

We show that the third-order optical response of disordered linear J-aggregates can be calculated by considering only a limited number of transitions between (multi-) exciton states. We calculate the pump-probe absorption spectrum resulting from the truncated set of transitions and show that, apart from the blue wing of the induced absorption peak, it agrees well with the exact spectrum.

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