Room- and low-temperature magnetic properties of 2-D magnetite particle arrays

Mathematics – Logic

Scientific paper

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Archaeomagnetism, Environmental Magnetism, Rock And Mineral Magnetism

Scientific paper

Palaeomagnetic observations are being used in increasingly sophisticated geological and geophysical interpretations. It is therefore important to test the theories behind palaeomagnetic recording by rocks, and this can only be achieved using samples containing precisely controlled magnetic mineralogy, grain size and interparticle spacing, the last of which controls the degree of magnetostatic interactions within the samples. Here we report the room- and low temperature magnetic behaviour of a set of samples produced by the nano-scale patterning technique electron beam lithography. The samples consist of 2-D arrays of near-identical magnetite dots of various sizes, geometries and spatial configurations, with dot sizes from ranging from near the single domain threshold of 74-333 nm. We have made a series of magnetic measurements including hysteresis, first-order-reversal curve measurements and remanence acquisition, many as a function of temperature between 20 and 300 K, to quantify the samples’ behaviour to routine palaeomagnetic measurement procedures. We have also examined the behaviour of saturation isothermal remanences (SIRM) to cooling and warming cycling of the sample below room temperature. In addition, we investigated the samples’ responses to alternating-field demagnetization of room temperature induced SIRM, anhysteretic remanent magnetization (ARM) and partial ARM. ARM was used as a non-heating analogue for natural thermoremanence. Given the 2-D spatial distribution of the samples, in all the experiments we conducted both in-plane and out-of-plane measurements. Generally, the samples were found to display pseudo-single-domain hysteresis characteristics, but were found to be reliable recorders of weak-field remanences like ARM. For the closely packed samples, the samples’ magnetic response was highly dependent on measurement orientation.

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