Revelation of the role of impurities and conduction electron density in the high resolution photoemission study of ferromagnetic hexaborides

Physics – Condensed Matter – Materials Science

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Scientific paper

10.1103/PhysRevLett.99.266401

We investigate the temperature evolution of the electronic structure of ferromagnetic CaB$_6$ using ultra-high resolution photoemission spectroscopy; electronic structure of paramagnetic LaB$_6$ is used as a reference. High resolution spectra of CaB$_6$ reveal finite density of states at the Fermi level, $\epsilon_F$ at all the temperatures and evidence of impurity induced localized features in the vicinity of $\epsilon_F$, which are absent in the spectra of LaB$_6$. Analysis of the high resolution spectra suggests that disorder in B-sublattice inducing partial localization in the mobile electrons and low electron density at $\epsilon_F$ is important to achieve ferromagnetism in these systems.

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