Physics – Condensed Matter – Materials Science
Scientific paper
2005-12-02
Phys. Rev. B 74, 020402 (R) (2006)
Physics
Condensed Matter
Materials Science
5 pages, 6 figures revised version
Scientific paper
10.1103/PhysRevB.74.020402
We show that resonant quantum tunneling of the magnetization, until now observed only in zero-dimensional (0D) cluster systems, occurs in the molecular Ising spin chain $[(CH_3)_3NH]CoCl_3\cdot 2H_2O$, which orders as a canted 3D-antiferromagnet at $T_C=4.15 K$. We present three features that prove unambigously the existence of resonant quantum tunneling below $0.3 K$ ($T_C/12$): Temperature independent relaxation of the magnetization, speeding up of the relaxation at a well defined field ($1025 Oe$) and increase of the magnetization each time this field is crossed during a succession of minor hysteresis loops. A mechanism is proposed to describe the behavior based on a simple model of 0D domain wall nucleation.
Khatsko E. N.
Lhotel Elsa
Paulsen Carley
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