Resonant Magnetization Tunneling in Mn12 Acetate: The Absence of Inhomogeneous Hyperfine Broadening

Physics – Condensed Matter – Mesoscale and Nanoscale Physics

Scientific paper

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Some minor revisions, title changed, updated figures, two added notes, one added reference. RevTeX, 4 pages, 3 postscript figu

Scientific paper

10.1103/PhysRevB.58.R14729

We present the results of a detailed study of the thermally-assisted-resonant-tunneling relaxation rate of Mn12 acetate as a function of an external, longitudinal magnetic field and find that the data can be fit extremely well to a Lorentzian function. No hint of inhomogeneous broadening is found, even though some is expected from the Mn nuclear hyperfine interaction. This inconsistency implies that the tunneling mechanism cannot be described simply in terms of a random hyperfine field.

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