Physics – Condensed Matter – Materials Science
Scientific paper
2010-01-08
Phys. Rev. Lett. 104, 037204 (2010)
Physics
Condensed Matter
Materials Science
Scientific paper
10.1103/PhysRevLett.104.037204
We show that low field magnetoelectric (ME) properties of helimagnets Ba0.5Sr1.5Zn2(Fe1-xAlx)12O22 can be efficiently tailored by Al-substitution level. As x increases, the critical magnetic field for switching electric polarization is systematically reduced from ~1 T down to ~1 mT, and the ME susceptibility is greatly enhanced to reach a giant value of 2.0 x 10^4 ps/m at an optimum x = 0.08. We find that control of nontrivial orbital moment in the octahedral Fe sites through the Al-substitution is crucial for fine tuning of magnetic anisotropy and obtaining the conspicuously improved ME characteristics.
Chai Yi Sheng
Chun Sae Hwan
Chung Jae-Ho
Haam So Young
Jaiswal-Nagar Deepshikha
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