Physics – Condensed Matter – Strongly Correlated Electrons
Scientific paper
2011-06-03
Phys. Rev. Lett. 107, 186405 (2011)
Physics
Condensed Matter
Strongly Correlated Electrons
A high-resolution version can be found at http://www.physics.ubc.ca/~quantmat/ARPES/PUBLICATIONS/Articles/BiSe_K.pdf
Scientific paper
The electronic structure of Bi2Se3 is studied by angle-resolved photoemission and density functional theory. We show that the instability of the surface electronic properties, observed even in ultra-high-vacuum conditions, can be overcome via in-situ potassium deposition. In addition to accurately setting the carrier concentration, new Rashba-like spin-polarized states are induced, with a tunable, reversible, and highly stable spin splitting. Ab-initio slab calculations reveal that these Rashba state are derived from the 5QL quantum-well states. While the K-induced potential gradient enhances the spin splitting, this might be already present for pristine surfaces due to the symmetry breaking of the vacuum-solid interface.
Butch Nicholas P.
Comin R.
Damascelli Andrea
Dosanjh P.
Elfimov I. S.
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