Quadrupolar Frustration in Shastry-Sutherland Lattice of DyB4 Studied by Resonant X-ray Scattering

Physics – Condensed Matter – Strongly Correlated Electrons

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5 pages, 4 figures, submitted to Physical Review Letter

Scientific paper

10.1143/JPSJ.74.2434

We have observed geometrical frustration of quadrupolar and magnetic moments in dysprosium tetraboride, DyB4, where the rare-earth sites form a Shastry-Sutherland lattice. Resonant x-ray scattering at the LIII absorption edge of Dy was utilized. Analysis of the energy, polarization, temperature, and azimuthal-angle dependences of the E1 resonance of the (1 0 0) forbidden reflection show that the magnetic and quadrupolar components within the frustrated c plane have a short-range correlation, suggesting that the moments are fluctuating. By contrast, the basic antiferromagnetic component along the c axis has a long-range order.

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