Physics – Condensed Matter – Strongly Correlated Electrons
Scientific paper
2010-01-28
Physics
Condensed Matter
Strongly Correlated Electrons
LA-UR 09-07829
Scientific paper
We report nonresonant inelastic x-ray scattering from the semi-core 5d levels of several actinide compounds. Dipole-forbidden, high-multipole features form a rich bound-state spectrum dependent on valence electron configuration and spin-orbit and Coulomb interactions. Cross-material comparisons, together with the anomalously high Coulomb screening required for agreement between atomic multiplet theory and experiment, demonstrate sensitivity to the neighboring electronic environment, such as is needed to address long-standing questions of electronic localization and bonding in 5f compounds.
Boland K. S.
Bradley Arthur J.
Clark David L.
Conradson Steven D.
Gupta Sanjib S.
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