Physics – Condensed Matter – Strongly Correlated Electrons
Scientific paper
2010-09-20
Physics
Condensed Matter
Strongly Correlated Electrons
10 pages, 4 figures
Scientific paper
The transient optical conductivity of photoexcited 1T-TaS2 is determined over a three-order-of-magnitude frequency range. Prompt collapse and recovery of the Mott gap is observed. However, we find important differences between this transient metallic state and that seen across the thermally-driven insulator-metal transition. Suppressed low-frequency conductivity, Fano phonon lineshapes, and a mid-infrared absorption band point to polaronic transport. This is explained by noting that the photo-induced metallic state of 1T-TaS2 is one in which the Mott gap is melted but the lattice retains its low-temperature symmetry, a regime only accessible by photo-doping.
Berger Helmuth
Cavalleri Andrea
Dean Nicky
Fausti Daniele
Gasparov Lev
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