Photoluminescence of single colour defects in 50 nm diamond nanocrystals

Physics – Condensed Matter – Materials Science

Scientific paper

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proceedings of ICDS 23 conference (23rd International Conference on Defects in Semiconductors, July 24 - July 29, 2005, Awaji

Scientific paper

10.1016/j.physb.2005.12.232

We used optical confocal microscopy to study optical properties of diamond 50 nm nanocrystals first irradiated with an electron beam, then dispersed as a colloidal solution and finally deposited on a silica slide. At room temperature, under CW laser excitation at a wavelength of 514.5 nm we observed perfectly photostable single Nitrogen-Vacancy (NV) colour defects embedded in the nanocrystals. From the zero-phonon line around 575 nm in the spectrum of emitted light, we infer a neutral NV0 type of defect. Such nanoparticle with intrinsic fluorescence are highly promising for applications in biology where long-term emitting fluorescent bio-compatible nanoprobes are still missing.

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