Phase Evolution of Solitonlike Optical Pulses during Excitonic Rabi Flopping in a Semiconductor

Physics – Condensed Matter

Scientific paper

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Time-Resolved Optical Spectroscopies And Other Ultrafast Optical Measurements In Condensed Matter, Optical Transient Phenomena: Quantum Beats, Photon Echo, Free-Induction Decay, Dephasings And Revivals, Optical Nutation, And Self-Induced Transparency, Exciton-Mediated Interactions, Theory, Models, And Numerical Simulation

Scientific paper

We demonstrate that the temporal pulse phase remains essentially unaltered before separate phase characteristics are developed when propagating high-intensity pulses coherently on the exciton resonance of an optically thick semiconductor. This behavior is a clear manifestation of self-induced transmission and pulse breakup into solitonlike pulses due to Rabi flopping of the carrier density. Experiments using a novel fast-scan cross-correlation frequency-resolved optical gating (XFROG) method are in good agreement with numerical calculations based on the semiconductor Bloch equations.

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