Oxygen stoichiometry, crystal structure, and magnetism in La$_{0.5}$Sr$_{0.5}$CoO$_{3-δ}$

Details Oxygen stoichiometry, crystal structure, and magnetism in La$_{0.5}$Sr$_{0.5}$CoO$_{3-δ}$ Oxygen stoichiometry, crystal structure, and magnetism in La$_{0.5}$Sr$_{0.5}$CoO$_{3-δ}$

2004-05-22

arxiv.org/abs/cond-mat/0405535v2

J. Phys. Condens. Matter 16 (2004) 6477-6484.

Physics

Condensed Matter

Materials Science

11 pages and 6 figures

Scientific paper

10.1088/0953-8984/16/36/013

We have prepared a series of polycrystalline samples La$_{0.5}$Sr$_{0.5}$CoO$_{3-\delta}$} with $0 < \delta \le 0.21$ and characterized their oxygen content, crystal structure, and magnetic properties. While the fully oxygenated samples are good ferromagnets, samples with larger $\delta$ values display increasingly broad magnetic transitions. The saturation magnetization at 5 K falls rapidly as $\delta$ increases. First principles electronic structure calculations provide insights into the magnetic behavior of the fully oxygenated compound, and the manner in which ferromagnetic ordering is affected by increasing oxygen non-stoichiometry.

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