Physics – Condensed Matter – Strongly Correlated Electrons
Scientific paper
2002-10-18
Physics
Condensed Matter
Strongly Correlated Electrons
4 pages, 4 figures
Scientific paper
10.1103/PhysRevLett.91.147205
55Mn and 139La NMR measurements on a high quality single crystal of ferromagnetic (FM) La0.80Ca20MnO3 demonstrate the formation of localized Mn(3+,4+) states below 70 K, accompanied with strong anomalous increase of certain FM neutron Bragg peaks. (55,139)(1/T1) spin-lattice relaxation rates diverge on approaching this temperature from below, signalling a genuine phase transition at T(tr) approx. 70 K. The increased local magnetic anisotropy of the low temperature phase, the cooling-rate dependence of the Bragg peaks, and the observed finite size scaling of T(tr) with Ca (hole) doping, are suggestive of freezing into an orbital domain state, precursor to a phase transition into an inhomogeneous orbitally ordered state embodying hole-rich walls.
Ansermet J.-Ph.
Belesi M.
Dimitropoulos C.
Dolinsek J.
Fardis M.
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