On the Tunneling Properties of non-Planar Molecules in a Gas Medium

Details On the Tunneling Properties of non-Planar Molecules in a Gas Medium On the Tunneling Properties of non-Planar Molecules in a Gas Medium

2011-10-14

arxiv.org/abs/1110.3285v1

Phys. Rev. A 84, 062115 (2011)

Physics

Condensed Matter

Statistical Mechanics

9 pages, 3 Figures

Scientific paper

10.1103/PhysRevA.84.062115

We propose a simple, general, and accurate formula for analyzing the tunneling between classical configurations of a non-planar molecule in a gas medium, as a function of the thermodynamic parameters of the gas. We apply it to two interesting cases: i) The shift to zero frequency of the inversion line of ammonia, upon increase of the pressure of the gas; ii) The destruction of the coherent tunneling of D2S2 molecules in a gas of He. In both cases, we compare our analysis with previous theoretical and experimental results.

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