On the Temperature Dependence of the Lifetime of Thermally Isolated Metastable Clusters

Details On the Temperature Dependence of the Lifetime of Thermally Isolated Metastable Clusters On the Temperature Dependence of the Lifetime of Thermally Isolated Metastable Clusters

2010-01-03

arxiv.org/abs/1001.0364v1

Phys. Solid State 52, 201 (2010)

Physics

Condensed Matter

Mesoscale and Nanoscale Physics

14 pages, 4 figures

Scientific paper

The temperature dependence of the lifetime of the thermally isolated metastable N8 cubane up to its decay into N2 molecules has been calculated by the molecular dynamics method. It has been demonstrated that this dependence significantly deviates from the Arrhenius law. The applicability of the finite heat bath theory to the description of thermally isolated atomic clusters has been proved using statistical analysis of the results obtained.

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