Physics – Condensed Matter – Mesoscale and Nanoscale Physics
Scientific paper
2009-10-06
Phys. Rev. Lett. 103, 197202 (2009)
Physics
Condensed Matter
Mesoscale and Nanoscale Physics
4 pages, 3 figures, with supplementary information file (3 pages, 3 figures). Minor corrections in V2, as published
Scientific paper
We present the first quantitative experimental evidence for the underscreened Kondo effect, an uncomplete compensation of a quantized magnetic moment by conduction electrons, as originally proposed by Nozieres and Blandin. The device consists of an even charge spin S = 1 molecular quantum dot, obtained by electromigration of C60 molecules into gold nanogaps and operated in a dilution fridge. The persistence of logarithmic singularities in the low temperature conductance is demonstrated by a comparison to the fully screened configuration obtained in odd charge spin S = 1/2 Coulomb diamonds. We also discover an extreme sensitivity of the underscreened Kondo resonance to magnetic field, that we confirm on the basis of numerical renormalization group calculations.
Balestro Franck
Costi Theo A.
Florens Serge
Roch Nicolas
Wernsdorfer Wolfgang
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